There's another, similar and current thread on this topic:
https://www.winnieowners.com/forums/...ml#post3924843
There are numerous Youtube reviews comparing the amp output of different portable solar panels and they're battery charging capabilities. The main variable for you is how many amp hours do you use in a day.
To answer a couple of your questions:
1. Pre-wired for solar doesn't include a controller. Many portable units come complete with controller but see the above thread for more info on the advantages and disadvantages of a built-in or seperate controller.
2. A lithium, or more specifically a LiFePO4 (Lithium Iron Phosphate Battery) can definitely be a plus, more usable amp hours, faster charging, etc. but I wouldn't put it at the top of my list. You will need to educate yourself a lot before taking this leap and isn't essential. I'd add a second battery similar to what you have and see what that looks like. If, by "deep cycle" battery, you mean the typical, dual purpose, flooded RV/Marine battery commonly installed on RVs, I'd replace it with two AGM deep cycle batteries. Keep in mind, however, that more battery capacity will increase the charging time.
For less than $32 more than the Jackery 100W panel, Renogy has a 200W solar suitcase for $330 with controller:
https://www.amazon.com/Renogy-200-Wa...sr=1-1-catcorr
Personally, I'd go with a combination of rooftop and portable panels. Portable panels have their advantages but there is the risk of theft. I wouldn't want to leave them unattended for long periods of time.